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81.
《环境科学学报(英文版)》2023,35(4):697-707
Indoor particle release from toner printing equipment (TPE) is a major health concern and has received wide attention. In this study, nine printing centers were randomly selected and three working phases were simulated, namely, non-working, normal printing/copying, and heavy printing/copying. The dynamics of the ozone (O3), volatile organic compound (VOC), and particle emissions from TPE were determined by portable detectors. Results showed that particles, VOCs, and O3 were indeed discharged, and particles and VOCs concentrations remained at high levels. Among them, 44% of the rooms represented high-level particle releases. Submicrometer-sized particles, especially nanoparticles, were positively correlated with VOCs, but were inversely proportional to the O3 concentration. Four elements, Ca, Al, Mg and Ni, were usually present in nanoparticles because of the discharge of paper. Si, Al, K, Ni and Pb were found in the submicrometer-sized particles and were consistent with the toner composition. The potential particle precursors were identified, which suggested that styrene was the most likely secondary organic aerosol (SOA) precursor. Overall, the use of the toner formulation and the discharge of paper attribute to the TPE-emitted particles, in which styrene is a specific monitoring indicator for the formation of SOA. 相似文献
82.
颗粒物是我国大多数城市环境空气中的首要污染物.由于缺乏对颗粒物成分及来源的研究,导致目前的控制措施常常缺乏针对性.为全面弄清城市环境空气中颗粒物的来源,分采暖期和非采暖期对城市的主要大气污染源进行识别和采样,包括煤烟尘、建筑水泥尘、扬尘、土壤风沙尘、海盐粒子和二次粒子,并利用原子发射光谱、离子色谱等仪器对其成分进行定性定量分析,建立可吸入颗粒物的源成分谱.从而得出颗粒物元素成分谱,通过化学质量平衡(CMB)受体模型进行解析,得出各污染源对受体的贡献值和分担率.确定主要污染源,为采取针对性的措施治理污染提供依据. 相似文献
83.
84.
1987-1989年春秋季在西南重庆、贵阳、成都和广元等地区采集大气颗粒物和雨水样品,测定了其中S和SO4^2-。探讨了颗粒物中S在粗细粒中的分布及水溶性S的百分比,估算了大气中S在气相(SO2)、液相(H2SO4)及固相(SO4^2-)中的分配比例,得知颗粒物中S对降雨的贡献率为18~50%。 相似文献
85.
H.A. Carreras M.L. Pignata P.H.N. Saldiva 《Atmospheric environment (Oxford, England : 1994)》2006,40(40):7824-7830
During the last decades, a significant deterioration of ambient air quality has been observed in Argentina. However, the availability of air pollution monitoring stations is still limited to only few cities. In this study, we investigated the genotoxicity of ambient levels of air pollution in Córdoba using the Tradescantia micronucleus assay. The experiment was performed from October, 2004 to April 2005. Pots with Tradescantia pallida were placed in three sites: Córdoba city center, characterized by important avenues with high traffic activity (cars, taxis, and public transport vehicles); the university campus, along a side road with heavy traffic of gasoline and diesel powered vehicles, buses and trucks; and a residential area, with no significant local sources of air pollution. Twenty young T. pallida inflorescences were collected from each sampling site in November, February and April. Micronuclei frequencies were determined in early tetrads of pollen mother cells and expressed as MCN/100 tetrads. Simultaneously, the environmental levels of total suspended particles (24 h mean) were determined for each site. A significant difference in micronuclei frequency was observed among sites (p=0.036). Post-hoc analysis revealed that the residential area exhibited a lower micronuclei frequency than the university and city center areas. In conclusion, we found that the gradients of ambient air pollution of Córdoba are associated with changes in the spontaneous micronuclei frequency of Tradescantia pollen mother cells. These results indicate that in situ biomonitoring with higher plants may be useful for characterizing air pollution in areas without instrumental monitoring techniques, or for exploring the distribution of air contaminants at a microscale. 相似文献
86.
Composition of torched crude oil organic particulate emitted by refinery and its similarity to atmospheric aerosol in the surrounding area 总被引:3,自引:0,他引:3
The absolute contents and relative distributions of organic aerosols [n-alkanes, n-alkanoic and n-alkenoic acids, n-alkan-2-ones and polycyclic aromatic hydrocarbons (PAH)] were determined in torched gases emitted during the crude oil extraction and in the free atmosphere of the Hassi-Messaoud city (Algeria). Monocarboxylic acids, both saturated and monounsaturated (from 9802 to 20 057 ng m−3), accounted for the major fraction of the total particulate organic matter identified both in torch exhaust and atmospheric particulate. n-Alkanes were also abundant both in the direct emission (from 460 to 632 ng m−3) and city atmosphere (462 ng m−3) and displayed a peculiar fingerprint characterised by the presence of a set of branched congeners around even carbon-numbered homologues and a strong even-to-odd predominance along the whole carbon number range (C16–C34). Whilst n-alkan-2-ones were absent in the city and poor in smokes emitted from the torches (from 31 to 42 ng m−3), PAH were present at low extents in all sites (from 18 to 65 ng m−3). The incomplete thermal combustion of torched crude oil was very likely the main source of these particle-bound organic constituents in the city and its surrounding region. 相似文献
87.
R. Vautard P. Ciais R. Fisher D. Lowry F.M. Bron F. Vogel I. Levin F. Miglietta E. Nisbet 《Atmospheric environment (Oxford, England : 1994)》2007,41(40):9506-9517
The dispersion of pollutants from the huge Buncefield oil depot fire that occurred on 11 December 2005 is simulated using a regional Eulerian chemistry-transport model. We analyse the transport and mixing of the fire plume. We show that the hot plume never reached the ground. Instead, it pierced the thin wintertime boundary layer and was injected into the free troposphere at higher altitudes. This is in agreement with data from many air quality stations. This high injection was fortunate because the fine aerosol particles (PM10) mass column generated by the fire smoke exceeded that of ordinary pollution by an order of magnitude. Our regional chemistry-transport modelling is able to predict the early development of the plume dispersion, as shown by a qualitative comparison between simulated PM10 columns and a satellite image obtained by the EOS-TERRA-MODIS sensor.If the accident had occurred in summer when boundary layers are much deeper and convective, a severe degradation in air quality due to PM10 could have occurred, as shown by a sensitivity simulation assuming a similar fire during one of the hottest days of August 2003. The modelled impact of the fire on regional and European air quality levels strongly depends on the altitude reached by the buoyant plume, as shown by a set of sensitivity simulations with variable injection heights. However, in all cases we found that the fire only affected surface aerosol concentrations without increasing photochemical pollution. 相似文献
88.
Particulate air pollution in Lanzhou China 总被引:4,自引:0,他引:4
Concentrations of total suspended particles (TSP) and PM(10) in Lanzhou China have been kept high for the past two decades. Data collected during the intensive observational period from October 1999 to April 2001 show high TSP and PM(10) concentrations. Starting from November, the PM(10) pollution intensifies, and reaches mid to high alert level of air pollution, continues until April next year, and is at low alert level in the summer. In the winter and spring, the TSP concentration is 2-10 times higher than the third-level criterion of air quality (severe pollution). Effects of intrinsic factors (sources of pollution) and remote preconditions (propagation of dust storms) for severe PM(10) and TSP pollution in Lanzhou are analyzed. 相似文献
89.
This paper investigates the effect of low emission zones on air quality and birth outcomes in Germany. The staggered introduction of the policy measure creates a credible natural experiment and a natural control group for births and air pollution measurements in cities that enact low emission zones. I show that the introduction of the most restrictive type of low emission zone decreases average levels of fine particulate matter by about 4 percent and by up to 8 percent at a city's highest-polluting monitor. Low emission zones also reduce the number of days per year on which legal pollution limits are exceeded by three. However, these reductions are too small to translate into substantial improvements in infant health. My results are not driven by changes in maternal or city specific characteristics, and are robust to variations in specification and to the choice of control group. 相似文献
90.
Aatmeeyata D.S. Kaul Mukesh Sharma 《Atmospheric environment (Oxford, England : 1994)》2009,43(35):5691-5697
This study aimed to understand the non-exhaust (NE) emission of particles from wear of summer tire and concrete pavement, especially for two wheelers and small cars. A fully enclosed laboratory-scale model was fabricated to simulate road tire interaction with a facility to collect particles in different sizes. A road was cast using the M-45 concrete mixture and the centrifugal casting method. It was observed that emission of large particle non exhaust emission (LPNE) as well as PM10 and PM2.5 increased with increasing load. The LPNE was 3.5 mg tire−1 km−1 for a two wheeler and 6.4 mg tire−1 km−1 for a small car. The LPNE can lead to water pollution through water run-off from the roads. The contribution of the PM10 and PM2.5 was smaller compared to the LPNE particles (less than 0.1%). About 32 percent of particle mass of PM10 was present below 1 μm. The number as well as mass size distribution for PM10 was observed to be bi-modal with peaks at 0.3 μm and 4–5 μm. The NE emissions did not show any significant trend with change in tire pressure. 相似文献